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N- to C-sulfonyl photoisomerisation of dihydropyridinones: a synthetic and mechanistic study

The scope and limitations of a photoinitiated N- to C-sulfonyl migration process within a range of dihydropyridinones is assessed. This sulfonyl transfer proceeds without erosion of either diastereo- or enantiocontrol, and is general across a range of N-sulfonyl substituents (SO2R; R = Ph, 4-MeC6H4, 4-MeOC6H Mechanistic Aspects of Organic Synthesis

Authors:   Pei-Pei Yeh; James E. Taylor; Daniel G. Stark; David S. B. Daniels; Charlene Fallan; John C. Walton; Andrew D. Smith
Journal:   Organic & Biomolecular Chemistry
Volume:   15
edition:   42
Pages:   8914
DOI:   10.1039/C7OB01699A
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