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Probing of Field-Induced Structures and Their Dynamics in Ferrofluids Using Oscillatory Rheology

10-10-2014 | Leona J. Felicia; John Philip, Langmuir, 2014

We probe field-induced structures and their dynamics in ferrofluids using oscillatory rheology. The magnetic field dependence of the relaxation time and crossover modulus showed two distinct regions, indicating the different microstructures in those regions. The observed relaxation at various ...


Ionic Liquids Entrapped in Reverse Micelles as Nanoreactors for Bimolecular Nucleophilic Substitution Reaction. Effect of the Confinement on the Chloride Ion Availability

10-10-2014 | Diana Blach; Marcia Pessêgo; Juana J. Silber; N. Mariano Correa; Luis García-Río; R. Darío Falcone, Langmuir, 2014

In this work was explored how the confinement of two ionic liquids (ILs), 1-butyl-3-methylimidazolium chloride (bmimCl) and 1-butyl-3-methylimidazolium tetrafluoroborate (bmimBF4), inside toluene/benzyl-n-hexadecyldimethylammonium chloride (BHDC) reverse micelles (RMs) affects the Cl– ...


Eliminating the Roughness in Cholesterol’s β-Face: Does it Matter?

10-10-2014 | Martin R. Krause; Minghui Wang; Laurel Mydock-McGrane; Douglas F. Covey; Emmanuel Tejada; Paulo F. Almeida; Steven L ..., Langmuir, 2014

One of the long-standing issues surrounding cholesterol (Chol) relates to its two-faced character. In particular, the consequences of its having a rough β-face and a smooth α-face on its structural influence in cell membranes has remained elusive. In this study, direct comparisons have been made ...


[70]Fullerenes Assist the Formation of Phospholipid Bicelles at Low Lipid Concentrations

10-10-2014 | Atsushi Ikeda; Kazuya Kiguchi; Tomohiro Hida; Kazuma Yasuhara; Kazuyuki Nobusawa; Motofusa Akiyama; Wataru Shinoda, Langmuir, 2014

Langmuir DOI: 10.1021/la503732q


Tailoring the Hydrophilic/Lipophilic Balance of Clickable Mesoporous Organosilicas by the Copper-Catalyzed Azide–Alkyne Cycloaddition Click-Functionalization

09-10-2014 | Achraf Noureddine; Philippe Trens; Guillaume Toquer; Xavier Cattoën; Michel Wong Chi Man, Langmuir, 2014

We have designed and synthesized a clickable bridged silsesquioxane material featuring pendant alkyne chains as an aggregate of golf-ball-like nanoparticles, as evidenced by scanning electron microscopy (SEM), transmission electron microscopy (TEM), and small- and wide-angle X-ray scattering ...


Investigation of the Sodium Ion Pathway and Cathode Behavior in Na3V2(PO4)2F3 Combined via a First Principles Calculation

09-10-2014 | Weixin Song; Xiaoyu Cao; Zhengping Wu; Jun Chen; Yirong Zhu; Hongshuai Hou; Qing Lan; Xiaobo Ji, Langmuir, 2014

The electrochemical properties of Na3V2(PO4)2F3 cathode utilized in the sodium ion battery are investigated, and the ion migration mechanisms are proposed as combined via the first principles calculations. Two different Na sites, namely, the Na(1) and Na(2) sites, could cause two sodium ions of ...


Microfluidic Production of Perfluorocarbon-Alginate Core–Shell Microparticles for Ultrasound Therapeutic Applications

09-10-2014 | Ana Rita C. Duarte; Barış Ünal; João F. Mano; Rui L. Reis; Klavs F. Jensen, Langmuir, 2014

The fabrication of micrometer-sized core–shell particles for ultrasound-triggered delivery offers a variety of applications in medical research. In this work, we report the design and development of a glass capillary microfluidic system containing three concentric glass capillary tubes for the ...


Use of Eutectic Mixtures for Preparation of Monolithic Carbons with CO2-Adsorption and Gas-Separation Capabilities

09-10-2014 | N. López-Salas; E. O. Jardim; A. Silvestre-Albero; M. C. Gutiérrez; M. L. Ferrer; F. Rodríguez-Reinoso; J. Silvestre ..., Langmuir, 2014

With global warming becoming one of the main problems our society is facing nowadays, there is an urgent demand to develop materials suitable for CO2 storage as well as for gas separation. Within this context, hierarchical porous structures are of great interest for in-flow applications because ...


On-Demand Droplet Fusion: A Strategy for Stimulus-Responsive Biosensing in Solution

09-10-2014 | Praveena Mohan; Patrick S. Noonan; Matthew A. Nakatsuka; Andrew P. Goodwin, Langmuir, 2014

A novel strategy is reported for biochemically controlled fusion of oil-in-water (O/W) droplets as an in-solution sensor for biological targets. Inspired by the SNARE complex in cells, the emulsions were stabilized by a combination of phospholipids, phospholipid–poly(ethylene glycol) conjugates, ...


Light-Responsive Smart Surface with Controllable Wettability and Excellent Stability

09-10-2014 | Yin-Ning Zhou; Jin-Jin Li; Qing Zhang; Zheng-Hong Luo, Langmuir, 2014

Novel fluorinated gradient copolymer was designed for smart surface with light-responsive controllable wettability and excellent stability. The switchable mechanism and physicochemical characteristics of the as-prepared surface decorated by designed polymeric material were investigated by ...


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