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Effect of alkyl chain length of tri-n-alkyl phosphate extractants on the electrochemical behaviour of U(VI) in ionic liquid medium

25-Apr-2016 | Author(s): R. Rama, Alok Rout, K.A. Venkatesan, M.P. Antony, Journal of Electroanalytical Chemistry, 2016

Publication date: 15 June 2016 Source:Journal of Electroanalytical Chemistry, Volume 771 Author(s): R. Rama, Alok Rout, K.A. Venkatesan, M.P. Antony Higher homologs of trialkyl phosphates have been proposed for the separation of U(VI) from fast reactor dissolver solution by liquid – ...


Covariance‐Based Hardware Selection Part IV: Solution Using the Generalized Benders Decomposition

22-Apr-2016 | Jin Zhang, Xiaoxi Wang, Donald J. Chmielewski, AIChE Journal, 2016

Abstract Recently the covariance based hardware selection problem has been shown to be of the Mixed Integer Convex Programming (MICP) class. While such a formulation provides a route to global optimality, use of the branch and bound search procedure has limited application to fairly small ...


Molybdenum–Bismuth Bimetallic Chalcogenide Nanosheets for Highly Efficient Electrocatalytic Reduction of Carbon Dioxide to Methanol

21-Apr-2016 | Xiaofu Sun, Qinggong Zhu, Xinchen Kang, Huizhen Liu, Qingli Qian, Zhaofu Zhang, Buxing Han, Angewandte Chemie International Edition, 2016

Abstract Methanol is a very useful platform molecule and liquid fuel. Electrocatalytic reduction of CO2 to methanol is a promising route, which currently suffers from low efficiency and poor selectivity. Herein we report the first work to use a Mo‐Bi bimetallic chalcogenide (BMC) as an ...


Oxygen Reduction Reaction on Graphene in an Electro‐Fenton System: In Situ Generation of H2O2 for the Oxidation of Organic Compounds

21-Apr-2016 | Chen‐Yu Chen, Cheng Tang, Hao‐Fan Wang, Cheng‐Meng Chen, Xiaoyuan Zhang, Xia Huang, Qiang Zhang, ChemSusChem, 2016

Abstract Fenton oxidation using an aqueous mixture of Fe2+ and H2O2 is a promising environmental remediation strategy. However, the difficulty of storage and shipment of concentrated H2O2 and the generation of iron sludge limit its broad application. Therefore, highly efficient and ...


Investigating the effect of flexible constraints on the accuracy of self‐modeling curve resolution methods in the presence of perturbations

21-Apr-2016 | Nahal Rahimdoust Mojdehi, Mathias Sawall, Klaus Neymeyr, Hamid Abdollahi, Journal of Chemometrics, 2016

Self‐modeling curve resolution methods have continuously been improved during recent years. Many efforts have been made on curve resolution methods to reduce the rotational ambiguity by means of different types of constraints. Choosing proper constraints and cost functions is critically ...


Polyvinylferrocene-Based Amphiphilic Block Copolymers Featuring Functional Junction Points for Cross-Linked Micelles

21-Apr-2016 | Jan Morsbach; Johannes Elbert; Christian Rüttiger; Svenja Winzen; Holger Frey; Markus Gallei, Macromolecules, 2016

The synthesis of high-molecular-weight, well-defined poly(vinylferrocene)-block-poly(ethylene glycol) (PVFc-b-PEG) diblock copolymers (Mn = 13 000–44 000 g mol–1; Đ = 1.29–1.34) with precisely one allyl group at the junction point is introduced. Allyl glycidyl ether (AGE) was used to ...


The electrochemical behavior of tellurium on stainless steel substrate in alkaline solution and the illumination effects

17-Apr-2016 | Author(s): Yanyun Fan, Liangxing Jiang, Jia Yang, Yan Jiang, Fangyang Liu, Journal of Electroanalytical Chemistry, 2016

Publication date: 15 June 2016 Source:Journal of Electroanalytical Chemistry, Volume 771 Author(s): Yanyun Fan, Liangxing Jiang, Jia Yang, Yan Jiang, Fangyang Liu The electrochemical behavior of tellurium on stainless steel plate substrate in alkaline solution and the illumination ...


Amino‐Functional Polybenzimidazole Blends with Enhanced Phosphoric Acid Mediated Proton Conductivity as Fuel Cell Electrolytes

15-Apr-2016 | David Aili, Irakli Javakhishvili, Junyoung Han, Katja Jankova, Chao Pan, Søren Hvilsted, Jens Oluf Jensen, Niels J. ..., Macromolecular Chemistry and Physics, 2016

A new amino‐functional polybenzimidazole copolymer is synthesized by homogeneous solution condensation polymerization from a novel monomer, N,N′‐bis(2,4‐diaminophenyl)‐1,3‐diaminopropane. The copolymer readily dissolves in organic solvents and shows good film forming characteristics. To balance ...


Nanostructure Restoration of Thermally Reduced Graphene Oxide Electrode upon Incorporation of Nafion for Detection of Trace Heavy Metals in Aqueous Solution

14-Apr-2016 | Pui Mun Lee, Hai Woon Ng, Ju Dy Lim, Nay Win Khun, Zhong Chen, Erjia Liu, Electroanalysis, 2016

Abstract High performance reduced graphene oxide (RGO)‐Nafion (N) thin film electrodes coated on silicon (Si) substrates (RGO‐N/Si) were successfully developed through thermal reduction of GO‐N without delamination from the substrates. The restoration of the RGO‐N nanostructure upon the ...


A Convenient Enantioselective CBS-Reduction of Arylketones in Flow-Microreactor Systems

13-Apr-2016 | sonia deangelis; Maddalena De Renzo; Claudia Carlucci; Leonardo Degennaro; RENZO LUISI, Organic & Biomolecular Chemistry, 2016

A convenient, versatile, and green CBS-asymmetric reduction of aryl and heteroaryl ketones has been developed by using the microreactor technology. The study demonstrates that it is possible to handle safely the borane solution within microreactors and that the reaction performs well using ...


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