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A chemical method for stabilizing a new series of solid solution in Pr1-xCexScO3 (0.0 [less-than-or-equal] x [less-than-or-equal] 1.0) system

02-Sep-2015 | Farheen N Sayed; Rakesh R Shukla; A. K. Tyagi, Dalton Transactions, 2015

A new series of Pr1-xCexScO3 (0.0 ≤ x ≤ 1.0) compounds was synthesized by a two-step synthesis route, involving combustion reaction followed by reduction while heating in low partial pressure of O2, generated by zirconium sponge that acts as an oxygen getter. For the first time, a perovskite ...

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Highly efficient visible-light-driven CO2 reduction to CO using a Ru(II)–Re(I) supramolecular photocatalyst in an aqueous solution

02-Sep-2015 | Akinobu Nakada; Kazuhide Koike; Kazuhiko Maeda; Osamu Ishitani, Green Chemistry, 2015

In an aqueous solution, [Ru(dmb)2-(BL)–Re(CO)3Cl]2+ (BL = bridging ligand) most efficiently photocatalyzed reduction of CO2 to CO under visible-light irradiation using 2-(1,3-dimethyl-2,3-dihydro-1H-benzimidazol-2-yl)benzoic acid (BI(CO2H)H) as a water-soluble sacrificial reductant (ΦCO = 13%, ...

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Photo-induced redox catalysis for proton reduction to hydrogen with homogeneous molecular systems using rhodium-based catalysts

30-Aug-2015 | Author(s): Thibaut Stoll, Carmen E. Castillo, Megumi Kayanuma, Martina Sandroni, Chantal Daniel, Fabrice ..., Coordination Chemistry Reviews, 2015

Publication date: 1 December 2015 Source:Coordination Chemistry Reviews, Volumes 304–305 Author(s): Thibaut Stoll, Carmen E. Castillo, Megumi Kayanuma, Martina Sandroni, Chantal Daniel, Fabrice Odobel, Jérôme Fortage, Marie-Noëlle Collomb Solar driven water-splitting into ...

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Surface Modification on Poly(ether ether ketone) with Phospholipid Polymer via Photoinduced Self‐Initiated Grafting

25-Aug-2015 | Kazuhiko Ishihara, Yuuki Inoue, Masayuki Kyomoto, Macromolecular Symposia, 2015

Summary A new and safer method for constructing a nanometer‐scale modified surface on the poly(ether ether ketone) (PEEK) is examined by “photoinduced self‐initiated graft polymerization”. The generation of semi‐benzopinacol‐containing radicals of the benzophenone units in PEEK molecular ...

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Refinement of the inversion‐transfer NMR experiment for faster characterization of chemical exchange

25-Aug-2015 | Evelyne Baguet, Magnetic Resonance in Chemistry, 2015

It is shown theoretically that the inversion‐transfer experiment used to estimate the value of unidirectional rate constants in chemical exchange systems can be performed faster via a reduction of the recovery delay. The chemical exchange rate constants can then be estimated accurately with a ...

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Manganese oxide nanoparticles/reduced graphene oxide as novel electrochemical platform for immobilization of FAD and its application as highly sensitive persulfate sensor

24-Aug-2015 | Samira Mansouri Majd, Abdollah Salimi, Bandar Astinchap, Electroanalysis, 2015

Abstract In this study, manganese oxide nanoparticles/reduced graphene oxide(MnOxNPs/rGO) was used as support for strong immobilization of flavin adenine dinucleotide(FAD). A thin film of rGO cast on the electrode surface, followed by performing electrodeposition of MnOxNPs at applied constant ...

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IJMS, Vol. 16, Pages 20050-20066: Development of a New Monomer for the Synthesis of Intrinsic Antimicrobial Polymers with Enhanced Material Properties

24-Aug-2015 | Brodkorb, Florian ; Fischer, Björn ; Kalbfleisch, Katrin ; Robers, Oliver ; Braun, Carina ; Dohlen, Sophia ; Kreyens ..., International Journal of Molecular Sciences, 2015

The use of biocidal compounds in polymers is steadily increasing because it is one solution to the need for safety and hygiene. It is possible to incorporate an antimicrobial moiety to a polymer. These polymers are referred to as intrinsic antimicrobial. The biocidal action results from contact ...

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A Polymer-Brush-Based Nanovalve Controlled by Nanoparticle Additives: Design Principles

21-Aug-2015 | Rob D. Coalson; Afshin Eskandari Nasrabad; David Jasnow; Anton Zilman, Journal of Physical Chemistry B, 2015

Polymer-grafted surfaces and channels are increasingly used for the design of responsive materials and sensors due to robust performance and ease of use. Various strategies for the control of the nanoscale morphologies of such materials and devices are being tested. Entropic repulsion between the ...

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Image signal‐to‐noise ratio estimation using adaptive slope nearest‐neighbourhood model

20-Aug-2015 | K. S. SIM, V. TEH, Journal of Microscopy, 2015

Summary A new technique based on nearest neighbourhood method is proposed. In this paper, considering the noise as Gaussian additive white noise, new technique single‐image‐based estimator is proposed. The performance of this new technique such as adaptive slope nearest neighbourhood is ...

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Rhenium Complexes of Ligands Based on Stilbene – Synthesis, Characterization, ­Reactivity, and Conformational Analysis

19-Aug-2015 | Arantxa Pino‐Cuevas, Rosa Carballo, Luis Muñoz, Ezequiel M. Vázquez‐López, European Journal of Inorganic Chemistry, 2015

Abstract The imine ligand L1 was prepared by the reaction of 4‐amino‐4′‐(dimethylamino)stilbene and 2‐pyridinecarbaldehyde. The amine ligand L2 was obtained in good yield by the reduction of L1 with NaBH4. The complexes [ReX(CO)3(Ln)] (1a: X = Cl, n = 1; 1b: X = Br, n = 1; 2a: X = Cl, n = 2; ...

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