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All‐Iron Redox Flow Battery Tailored for Off‐Grid Portable Applications

20-Nov-2015 | Michael C. Tucker, Adam Phillips, Adam Z. Weber, ChemSusChem, 2015

Abstract An all‐iron redox flow battery is proposed and developed for end users without access to an electricity grid. The concept is a low‐cost battery which the user assembles, discharges, and then disposes of the active materials. The design goals are: (1) minimize upfront cost, ...


Dysprosium‐ and Ytterbium‐Based Complexes Involving Tetrathiafulvalene Derivatives Functionalised with 2,2′‐Bipyridine or 2,6‐Di(pyrazol‐1‐yl)‐4‐pyridine

19-Nov-2015 | Min Feng, Saskia Speed, Fabrice Pointillart, Bertrand Lefeuvre, Boris Le Guennic, Stéphane Golhen, Olivier Cador, La ..., European Journal of Inorganic Chemistry, 2015

Abstract Two new tetrathiafulvalene‐based ligands {L1 = 4,5‐bis[2,6‐di(pyrazol‐1‐yl)‐4‐pyridylmethylthio]‐4′,5′‐bis(methylthio)tetrathiafulvene, L3 = 4‐(4′‐methyl‐2,2′‐bypiridin‐4‐ylmethylthio)‐5‐(2‐cyanoethylthio)‐4′,5′‐ethylenedithiotetrathiafulvene} have been elaborated and four new ...


Preparation of a CuInS2 Nanoparticle Ink and Application in a Selenization‐Free, Solution‐Processed Superstrate Solar Cell

19-Nov-2015 | Amir Hossein Cheshme Khavar, Ali Reza Mahjoub, Fariba Tajabadi, Mehdi Dehghani, Nima Taghavinia, European Journal of Inorganic Chemistry, 2015

Abstract We report a study on chalcopyrite solar cells fabricated by low‐cost, nonvacuum, and selenization‐free methods. Superstrate‐type CuInS2 (CIS) thin‐film solar cells were prepared by sequential ink deposition. The CIS film was formed from a stable low‐carbon ink, which was synthesized ...


Secondary Sphere Hydrogen Bonding in Monocopper Complexes of Potentially Dinucleating Bis(carboxamide) Ligands

18-Nov-2015 | Benjamin D. Neisen, Pavlo V. Solntsev, Mohammad R. Halvagar, William B. Tolman, European Journal of Inorganic Chemistry, 2015

Abstract Reaction of a macrocyclic ligand precursor comprising two bis(carboxamido)pyridine units (H4L4) connected by ethylene linkers with NMe4OH and CuX2 (X = Cl, OAc, or OTf) yielded monocopper complexes [NMe4][(H2L4)Cu(X)] [X = Cl (3), OAc (4), or OH (5)], in contrast to the results of ...


Osmotic power production from seawater brine by hollow fiber membrane modules: Net power output and optimum operating conditions

18-Nov-2015 | Sui Zhang, Tai‐Shung Chung, AIChE Journal, 2015

Abstract This study analyzes the net energy output and optimum operating conditions for osmotic power generation from seawater brine based on the currently available hollow fiber membranes in the module scale. Factors that are influential on membrane performances, such as external ...


Exploration of Quenching Pathways of Multiluminescent Acenes Using the GRRM Method with the SF-TDDFT Method

13-Nov-2015 | Satoshi Suzuki; Satoshi Maeda; Keiji Morokuma, Journal of Physical Chemistry A, 2015

The quenching pathways were investigated for three types of multiluminescent acene derivatives, which show environment-dependent fluorescence. Spin–flip time dependent density functional theory (SF-TDDFT) combined with the Global Reaction Route mapping (GRRM) strategy is employed to locate ...


Oscillatory Changes of the Heterogeneous Reactive Layer Detected with the Motional Resistance during the Galvanostatic Deposition of Copper in Sulfuric Solution

13-Nov-2015 | Alejandro Cuenca; Jerónimo Agrisuelas; José J. García-Jareño; Francisco Vicente, Langmuir, 2015

Metallic copper was galvanostatically deposited on quartz|gold resonant electrodes by applying a constant current in a 0.5 M CuSO4/0.1 M H2SO4 aqueous solution. Galvanostatic copper deposition is one of the best methodologies to calibrate the electrochemical quartz crystal microbalances (EQCM), a ...


Enhancing hematite photoanode activity for water oxidation by incorporation of reduced graphene oxide

12-Nov-2015 | Saulo A Carminati, Flavio Leandro De Souza, Ana F Nogueira, ChemPhysChem, 2015

Two effective methods to prepare reduced graphene oxide (rGO)/hematite nanostructured photoanodes and their photoelectrochemical characterization towards water splitting reactions are presented in this work. First, graphene oxide (GO) was reduced to rGO using hydrazine in a basic solution ...


Solid-State and Solution Structures of Glycinimine-Derived Lithium Enolates

10-Nov-2015 | Kyoung Joo Jin; David B. Collum, Journal of the American Chemical Society, 2015

A combination of crystallographic, spectroscopic, and computational studies was applied to study the structures of lithium enolates derived from glycinimines of benzophenone and (+)-camphor. The solvents examined included toluene and toluene containing various concentrations of tetrahydrofuran, ...


Self‐Supported Cobalt Phosphide Mesoporous Nanorod Arrays: A Flexible and Bifunctional Electrode for Highly Active Electrocatalytic Water Reduction and Oxidation

06-Nov-2015 | Yun‐Pei Zhu, Yu‐Ping Liu, Tie‐Zhen Ren, Zhong‐Yong Yuan, Advanced Functional Materials, 2015

Water splitting for the production of hydrogen and oxygen is an appealing solution to advance many sustainable and renewable energy conversion and storage systems, while the key fact depends on the innovative exploration regarding the design of efficient electrocatalysts. Reported herein is the ...


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